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美國布魯克海文儀器公司>技術文章>測量應用案例-20220905

技術文章

測量應用案例-20220905

閱讀:325          發布時間:2022-9-22
 

文獻名:Interactions between carbon-based nanoparticles and steroid hormone micropollutants in water

 

 

作者 Minh Nhat NguyenaPeter Georg WeidlerbRuth SchwaigercAndrea Iris Schäfera

a Institute for Advanced Membrane Technology (IAMT), Hermann-von-Helmholtz-Platz 1, 76344, Eggenstein-Leopoldshafen, Germany

b Institute of Functional Interfaces (IFG), Hermann-von-Helmholtz-Platz 1, 76344, Eggenstein-Leopoldshafen, Germany

c Institute for Applied Materials (IAM), Hermann-von-Helmholtz-Platz 1, 76344, Eggenstein-Leopoldshafen, Germany1

 

 

摘要:The occurrence of micropollutants (MPs) including steroid hormones is a global environmental and health challenge. Carbon-based nanoparticles can be incorporated with water treatment processes to allow MP removal by adsorption. The aim was to compare the suitability of such nanoparticles (graphene, graphene oxide, carbon nanotubes and C60) to adsorb steroid hormones for later incorporation in membrane composites. All nanoparticles displayed fast kinetics; carbon nanotubes and graphene showed high adsorption capacities for hormones undeterminable in isotherm studies (over 10?mg/g). External surface adsorption appears to be the most prominent factor impacting adsorption performance. Structure, conformation, geometry and surface charge of nanoparticles can influence the accessibility of surface area through colloidal instability in aqueous solution. Mechanism inspection shows that adsorption initiates at long ranges (up to 10?nm) through hydrophobic and electrostatic interactions. At relatively short ranges (0.2–0.5?nm), adsorption is enhanced by π/π stacking, XH / π (X = C, O) interactions, van der Waals forces and hydrogen bonding. Both long- and short-range forces transporting hormones from the liquid bulk into the adsorbed phase could control the rate. With relatively short residence time required and high adsorption capacity, carbon nanotubes and graphene are promising for incorporation in a membrane composite.

 

關鍵詞:Static adsorptionCarbon nanotubeGrapheneFullereneWater treatment

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